Grantee Research Project Results
Publications Details for Grant Number R830898
Developing Functional Fe(0)-based Nanoparticles for In Situ Degradation of DNAPL Chlorinated Organic Solvents
RFA:
Environmental Futures Research in Nanoscale Science Engineering and Technology (2002)
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| Reference Type | Citation | Progress Report Year | Document Sources |
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| Abstract | Lowry GV, Phenrat T, Fagerlund F, Kim H-J, Illangasekare T, Tilton RD. Controlled placement of polyelectrolyte modified engineered nanomaterials in the subsurface: correlating modifier layer properties and geochemistry with mobility. Eos Transactions 2007;88(52). |
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| Article/Press Release | Borchardt JK. Small science may clean a big problem. The Christian Science Monitor, February 10, 2005. |
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| Article/Press Release | Goho A. Special treatment: tiny technology tackles mega messes. Science News 2005;167(17):266. |
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| Article/Press Release | Kalaugher L. Nanoparticles seek out solvents in groundwater. April 13, 2004. |
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| Article/Press Release | Lowry GV. Nanotechnology increases efficiency of environmental technologies. Groundwater Monitoring and Remediation, Summer 2004. |
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| Article/Press Release | Spice B. Tiny engineered particles could one day remove common pollutant. Pittsburgh Post Gazette, Science and Technology Section, April 1, 2004. |
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| Book Chapter | Lowry GV, Wiesner MR. Environmental considerations: occurrences, fate, and characterization of nanoparticles in the environment. In: Monteiro-Riviere NA, Tran CL, eds. Nanotoxicology: Characterization, Dosing and Health Effects. New York, NY: Informa Healthcare USA, Inc., 2007, pp. 369-390. |
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| Book Chapter | Lowry GV. Nanomaterials for groundwater remediation. In: Wiesner M, Bottero J-Y, eds. Environmental Nanotechnology: Applications and Impacts of Nanomaterials. New York, NY: McGraw-Hill, 2007, pp. 297-333. |
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| Journal Article | Liu Y, Majetich SA, Tilton RD, Sholl DS, Lowry GV. TCE dechlorination rates, pathways, and efficiency of nanoscale iron particles with different properties. Environmental Science & Technology 2005;39(5):1338-1345. |
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| Journal Article | Liu Y, Choi H, Dionysiou D, Lowry GV. Trichloroethene hydrodechlorination in water by highly disordered monometallic nanoiron. Chemistry of Materials 2005;17(21):5315-5322. |
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| Journal Article | Liu Y, Lowry GV. Effect of particle age (Fe0 content) and solution pH on NZVI reactivity: H2 evolution and TCE dechlorination. Environmental Science & Technology 2006;40(19):6085-6090. |
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| Journal Article | Liu Y, Phenrat T, Lowry GV. Effect of TCE concentration and dissolved groundwater solutes on NZVI-promoted TCE dechlorination and H2 evolution. Environmental Science & Technology 2007;41(22):7881-7887. |
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| Journal Article | Phenrat T, Saleh N, Sirk K, Tilton RD, Lowry GV. Aggregation and sedimentation of aqueous nanoscale zerovalent iron dispersions. Environmental Science & Technology 2007;41(1):284-290. |
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| Journal Article | Phenrat T, Saleh N, Sirk K, Kim H-J, Tilton RD, Lowry GV. Stabilization of aqueous nanoscale zerovalent iron dispersions by anionic polyelectrolytes: adsorbed anionic polyelectrolyte layer properties and their effect on aggregation and sedimentation. Journal of Nanoparticle Research 2008;10(5):795-814. |
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| Journal Article | Saleh N, Phenrat T, Sirk K, Dufour B, Ok J, Sarbu T, Matyjaszewski K, Tilton RD, Lowry GV. Adsorbed triblock copolymers deliver reactive iron nanoparticles to the oil/water interface. Nano Letters 2005;5(12):2489-2494. |
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| Journal Article | Saleh N, Sarbu T, Sirk K, Lowry GV, Matyjaszewski K, Tilton RD. Oil-in-water emulsions stabilized by highly charged polyelectrolyte-grafted silica nanoparticles. Langmuir 2005;21(22):9873-9878. |
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| Journal Article | Saleh N, Sirk K, Liu Y, Phenrat T, Dufour B, Matyjaszewski K, Tilton RD, Lowry GV. Surface modifications enhance nanoiron transport and NAPL targeting in saturated porous media. Environmental Engineering Science 2007;24(1):45-57. |
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| Journal Article | Saleh N, Kim H-J, Phenrat T, Matyjaszewski K, Tilton RD, Lowry GV. Ionic strength and composition affect the mobility of surface-modified Fe0 nanoparticles in water-saturated sand columns. Environmental Science & Technology 2008;42(9):3349-3355. |
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| Journal Article | Sarbu T, Lin K-Y, Ell J, Siegwart DJ, Spanswick J, Matyjaszewski K. Polystyrene with designed molecular weight distribution by atom transfer radical coupling. Macromolecules 2004;37(9):3120-3127. |
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| Patent/Patent Application | Majetich S, McHenry M, Artman J, Staley S. Magnetic metal or metal carbide nanoparticles and a process for forming same. 1995;(Patent no. 5,456,986) |
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| Patent/Patent Application | Majetich S, McHenry M, Scott JH, Brunsman E, Kirkpatrick S. Metal, alloy, or metal carbide nanoparticles and a process for forming same. 1996;(Patent no. 5,549,973) |
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| Patent/Patent Application | Majetich S, McHenry M, Artman J, Staley S. Process for forming nanoparticles. 1998;(Patent no. 5,783,263) |
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| Patent/Patent Application | Matyjaszewski K, Tsarevsky N. Polymerization process for ionic monomers. U.S. Patent No. 6,624,262, September 23, 2003. |
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| Patent/Patent Application | Matyjaszewski K, Kowalewski T, Lambeth DN, Spanswick J, Tsarevsky NV. Process for the preparation of nanostructured materials. U.S. Patent No. 7,056,455, June 6, 2006. |
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| Patent/Patent Application | Matyjaszewski K, Pakula T. Polymers, supersoft elastomers and methods for preparing the same. U.S. Patent No. 7,019,082, March 28, 2006. |
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| Presentation | Almusallam A, Sholl D. Brownian dynamics study of polymer-stabilized nanoparticles. Presented at the Midwest Thermodynamics and Statistical Mechanics Conference, Buffalo, NY, June 4, 2004. |
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| Presentation | Baumann T, Keller AA, Auset-Vallejo M, Lowry GV. Micromodel study of transport issues during TCE dechlorination by ZVI colloids. Presented at the AGU Fall Meeting, San Francisco, CA, December 5-9, 2005. |
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| Presentation | Fagerlund F, Phenrat T, Kim H-J, Illangesakera T, Lowry GV. Nanoscale zero-valent iron treatment of a DNAPL source zone in sandy soils. Presented at the SERDP Partners in Technology Meeting, Washington, DC, December 4-6, 2007. |
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| Presentation | Kim H-J, Saleh N, Phenrat T, Tilton RD, Fagerlund F, Illangasekare T, Lowry GV. Effect of pH, pore water velocity, grain size, and clay content on the transportability of surface-modified NZVI in saturated sand columns. Presented at the SERDP Partners in Technology Meeting, Washington, DC, December 4-6, 2007. |
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| Presentation | Liu Y, Lowry G, Majetich S. TCE dechlorination by iron nanoparticles: effect of the surface oxide layer growth on the TCE dechlorination rate. Presented at the American Chemical Society 35th Central Regional Meeting, Pittsburgh, PA, October 19-22, 2003. |
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| Presentation | Liu Y, Majetich SA, Tilton RD, Sholl DS, Lowry GV. Aqueous-phase TCE dechlorination by nanoscale Fe0 particles: effect of iron properties on reaction pathways and products formed. Presented at the 42nd Annual Pittsburgh-Cleveland Catalysis Society Meeting, Pittsburgh, PA, June 18, 2004. |
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| Presentation | Liu Y, Choi H, Dionysiou D, Lowry G. Particle-scale understanding of TCE hydrodechlorination in water by poorly ordered nanoiron. To be presented at the Environmental Chemistry Division, 230th American Chemical Society National Meeting, Washington, DC, August 28-September 1, 2005. |
R830898 (2004) |
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| Presentation | Lowry GV, Dufour B, Kim H, Liu Y, Majetich S, Matyjaszewski K, Phenrat T, Saleh N, Sirk K, Tilton R. Groundwater remediation using nanoparticles. Presented at the Franco-American Workshop: Nanotechnologies for a Sustainable Environment, Rice University, Houston, TX, December 15-16, 2005. |
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| Presentation | Lowry GV, Liu Y, Majetich S, Matyjaszewski K, Phenrat T, Saleh N, Sirk K, Dufour B, Tilton R, Lowry BV. Environmental nanotechnology: a block copolymer-based strategy delivers nanoiron to subsurface DNAPL. Presented at the Department of Civil Engineering, University of Minnesota, November 4, 2005. |
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| Presentation | Lowry GV, Phenrat T, Saleh N, Liu Y, Sirk K, Tilton R. Creating stable nanoiron suspensions for efficient subsurface delivery to DNAPL source zones. Presented at the SERDP Partners in Environmental Technology Technical Symposium & Workshop, Washington, DC, November 28-30, 2005. |
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| Presentation | Lowry GV. Nanoiron in the subsurface: how far will it go and how does it change? Presented at the U.S. EPA Workshop on Nanotechnology for Site Remediation, Department of Commerce, Washington, DC, October 20-21, 2005. |
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| Presentation | Lowry GV. Delivering polymer-modified Fe0 nanoparticles to subsurface chlorinated organic solvent DNAPL. Presented at the U.S. EPA Nanotechnology and the Environment: Applications and Implications Progress Review Workshop III, Washington, DC, October 26-28, 2005. |
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| Presentation | Lowry GV. Fate and transport of nanomaterials in the environment. Presented at Nanotoxicology 2006, Boston, MA, April 25, 2006. |
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| Presentation | Lowry GV. Surface-functionalized reactive nanoparticles for groundwater remediation. Presented at the Department of Civil and Environmental Engineering, University of Delaware, March 10, 2006. |
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| Presentation | Lowry GV, Saleh N, Sirk K, PhenratT, Dufour B, Matyjaszewski K, Tilton RD. Triblock copolymer coatings enhances nanoiron transport and localizes nanoiron at the DNAPL/water interface. Presented at the Division of Geochemistry, 231st ACS National Meeting, Atlanta, GA, March 26-30, 2006. |
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| Presentation | Lowry GV, Saleh N, Liu Y, Phenrat T, Sirk K, Dufour B, Sarbu T, Matyjaszewski K, Tilton R. Nanoiron treatment of DNAPL source zones: efficient delivery and DNAPL targeting. Presented at the Fifth International Conference on Remediation of Chlorinated and Recalcitrant Compounds, Monterey, CA, May 22-25, 2006. |
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| Presentation | Lowry GV, Saleh N, Phenrat T, Kim H-J, Sirk K, Tilton RD, Illangasekare T. Effects of polymeric surface coatings on NZVI mobility in saturated porous media and reactivity with TCE. Presented at the Partners in Environmental Technology Technical Symposium & Workshop, Washington, DC, November 28-30, 2006. |
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| Presentation | Lowry GV, Saleh N, Phenrat T, Liu Y, Kim H, Sirk K, Matyjaszewski K, Tilton R. Delivering polymer-modified Fe0 nanoparticles to subsurface chlorinated organic solvent DNAPL. Presented at the U.S. EPA Nanotechnology and the Environment: Applications and Implications Progress Review Workshop III, Washington, DC, November 8-9, 2006. |
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| Presentation | Lowry GV, Phenrat T, Schoenfelder D, Losi M, Yi J, Peck SA. NZVI treatability study for a TCE source area at Alameda Point, CA. Presented at the SERDP Partners in Technology Meeting, Washington, DC, December 4-6, 2007. |
R830898 (Final) |
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| Presentation | Lowry G, Liu Y, Majetich S. Factors affecting the reactivity, efficiency, and lifetime of iron nanoparticles for in situ degradation of TCE. Presented at the American Geophysical Union Fall Meeting 2003, San Francisco, CA, December 8-12, 2003. |
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| Presentation | Lowry G. Nanomaterials: novel applications for DNAPL and PCB impacted sites. Presented at the April meeting of the Three Rivers Chapter of the Academy of Certified Hazardous Materials Managers, Pittsburgh, PA, April 8, 2004. |
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| Presentation | Lowry G, Tilton R, Sholl D, Majetich S, Matyjaszewski K. Developing functional Fe0-based nanoparticles for in situ degradation of DNAPL chlorinated organic solvents. Presented at the 227th American Chemical Society National Meeting, Anaheim, CA, April 1, 2004. |
R830898 (2003) R830898 (2004) R830898 (2005) R830898 (Final) |
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| Presentation | Lowry G, Liu Y, Tilton R, Sholl D, Sirk K, Saleh N, Sarbu T, Majetich S, Matyjaszewski K. Developing functional Fe0-based nanoparticles for in situ degradation of DNAPL chlorinated organic solvents. Presented at the U.S. EPA 2004 Nanotechnology Science To Achieve Results (STAR) Progress Review Workshop-Nanotechnology and the Environment II, August 18-20, 2004. |
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| Presentation | Lowry G, Liu Y. Lifetime and reactivity of NZVI in groundwater. Presented at the Partners in Environmental Technology Technical Symposium & Workshop, Washington, DC, November 28-30, 2006. |
R830898 (2005) R830898 (Final) |
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| Presentation | Phenrat T, Kim H-J, Tilton R, Fagerlund F, Illangesakera T, Lowry GV. Polyelectrolyte-modified nanoscale zerovalent iron: characteristics of the adsorbed polyelectrolyte layer and their effects on dispersion stability and TCE dechlorination. Presented at the SERDP Partners in Technology Meeting, Washington, DC, December 4-6, 2007. |
R830898 (Final) |
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| Presentation | Saleh NB, Sirk K, Sarbu T, Lowry GV, Tilton RD, Matyjaszewski K, Redden G. Targeted delivery of nanoiron to the NAPL-water interface. Presented at the 79th ACS Colloid and Surface Science Symposium, Clarkson University, Potsdam, NY, June 12-15, 2005. |
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| Presentation | Saleh NB, Sirk K, Sarbu T, Tilton RD, et al. Transport and DNAPL targeting of polyelectrolyte- and surfactant-modified nanoiron. To be presented at the Environmental Chemistry Division, 230th American Chemical Society National Meeting, Washington, DC, August 28-September 1, 2005. |
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| Presentation | Saleh N, Matyjaszewski K, Tilton RD, Lowry GV. Long-range transport of polymer-modified nanoiron in saturated porous sand and real aquifer media. Presented at the 80th ACS Colloid and Surface Science Symposium, Boulder, CO, June 18-21, 2006. |
R830898 (2005) R830898 (Final) |
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| Presentation | Saleh N, Sirk K, Phenrat T, Liu Y, Dufour B, Matyjaszewski K, Tilton RD, Lowry GV. Surface modifications enhance colloidal iron transport and deliver them to the NAPL/water interface. Presented at the Division of Colloid and Surface Chemistry for the 232nd ACS National Meeting, San Francisco, CA, September 10-14, 2006. |
R830898 (2005) R830898 (Final) |
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| Presentation | Saleh N, Sirk K, Phenrat T, Matyjaszewski K, et al. Mobility and DNAPL targeting of polymer-modified NZVI for in situ reduction of DNAPL source areas. Presented at the First International Conference on Dense Nonaqueous Phase Liquid Characterization and Remediation, Pittsburgh, PA, September 25-28, 2006. |
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| Presentation | Sirk K, Saleh NB, Liu Y, Sarbu T, Almusallam AS, Lowry G, Matyjaszewski K, Majetich S, Sholl D, Tilton R. Development of polymer-modified nanoparticles for targeted delivery of remediation agents to DNAPL/water interfaces. Presented at the AICHE 2004 National Meeting, Austin, TX, November 7-12, 2004. |
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| Presentation | Sirk K, Saleh NB, Matyjaszewski K, Lowry GV, Tilton RD. Development of triblock copolymers as dispersants and interfacial delivery vehicles for reactive nanoparticulate iron. Presented at the AICHE Annual Meeting, Engineering Sciences and Fundamentals Division, Cincinnati, OH, October 30-November 4, 2005. |
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| Presentation | Sirk K, Saleh N, Kim H-J, Phenrat T, Sarbu T, Dufour B, Ok J, Matyjaszewski K, Lowry GV, Tilton RD. Nanoiron surface modification by amphiphilic triblock copolymers for enhanced stability, transportability and accumulation at the NAPL/water interface. Presented at the 80th ACS Colloid and Surface Science Symposium, Boulder, CO, June 18-21, 2006. |
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| Presentation | Tilton RD, Lowry GV, Matyjaszewski K, Saleh NB, Sirk K, Liu Y, Sarbu T, Dufour B, Ok J, Phenrat T, Kim H-J. Triblock copolymers as nanoparticulate iron targeted delivery vehicles for source-zone remediation of contaminated aquifers. Presented at the Division of Colloid and Surface Chemistry, 231st ACS National Meeting, Atlanta, GA, March 26-30, 2006. |
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| Presentation | Tilton R, Sirk K, Saleh N, Lowry G. Development of polymer-decorated nanoparticles for targeted delivery of remediation agents to the trichloroethylene/water interface. Presented at the 78th ACS Colloid and Surface Science Symposium, New Haven, CT, June 20-23, 2004. |
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| Proceedings | Liu Y, Choi H, Dionysiou D, Lowry GV. Particle-scale understanding of TCE hydrodechlorination in water by poorly ordered nanoiron. In: Proceedings of the Environmental Chemistry Division, 230th American Chemical Society National Meeting, Washington, DC, August 28-September 1, 2005. |
R830898 (2005) R830898 (Final) |
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| Proceedings | Liu Y, Phenrat T, Lowry GV. Effect of groundwater constituents on H2 evolution and TCE reduction by reactive Fe0/Fe-oxide nanoparticles. In: Proceedings of the Division of Environmental Chemistry for the 233rd ACS National Meeting, Chicago, IL March 25-29, 2007. |
R830898 (Final) |
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| Proceedings | Lowry GV. Developing functional Fe0-based nanoparticles for in situ degradation of DNAPL chlorinated organic solvents. In: Proceedings of the 2004 Nanotechnology Science To Achieve Results (STAR) Progress Review Workshop-Nanotechnology and the Environment II, Philadelphia, PA: U.S. Environmental Protection Agency, August 18-20, 2004, EPA/600/R-05/089, p. 11. |
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| Proceedings | Lowry GV, Liu Y. Comparative evaluation of the reactivity and efficiency of two types of nanoscale zero-valent iron for reductive dehalogenation of TCE DNAPL. In: Proceedings of the Environmental Chemistry Division, 228th American Chemical Society National Meeting, Philadelphia, PA, August 22-26, 2004, Vol. 44, No. 2, pp. 412-417. |
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| Proceedings | Lowry GV. Fate and transport of nanomaterials. In: Proceedings of the Nanotechnology and OSWER: New Opportunities and Challenges Workshop, U.S. Environmental Protection Agency, July 12-13, 2006. |
R830898 (Final) |
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| Proceedings | Lowry GV, Saleh NB, Sirk K, Phenrat T, Dufour B, Matyjaszewski K, Tilton RD. Effect of groundwater geochemistry on nanoiron transport in saturated porous media. In: Proceedings of the Environmental Chemistry Division, 231st American Chemical Society National Meeting, Atlanta, GA, March 26-30, 2006. |
R830898 (2005) R830898 (Final) |
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| Proceedings | Lowry GV, Liu Y. Effect of pH and aging on NZVI corrosion rate and reactivity with TCE. In: Proceedings of the Environmental Chemistry Division, 231st American Chemical Society National Meeting, Atlanta, GA, March 26-30, 2006. |
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| Proceedings | Lowry GV, Liu Y. Nanoiron: reactant or catalyst? In: Proceedings of the Division of Environmental Chemistry, 232nd American Chemical Society National Meeting, San Francisco, CA, September 10-14, 2006. |
R830898 (2005) R830898 (Final) |
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| Proceedings | Lowry GV. NZVI for groundwater remediation: the importance of surface coatings for mobility and targeting. In: Proceedings of the EPA Region 5 Nanotechnology for Site Remediation Workshop, US EPA Region 5, Chicago, IL, September 6-7, 2006. |
R830898 (2005) R830898 (Final) |
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| Proceedings | Lowry GV. Delivering polymer-modified Fe0 nanoparticles to subsurface chlorinated organic solvent DNAPL. In: Proceedings of the U.S. Environmental Protection Agency Nanotechnology and the Environment: Applications and Implications Progress Review Workshop III, Washington, DC, October 26-28, 2005, pp. 44-48. |
R830898 (2005) |
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| Proceedings | Lowry GV. Environmental fate and transport of nanomaterials. In: Proceedings of the Nanotechnology and the Office of Solid Waste and Emergency Response: New Opportunities and Challenges, U.S. Environmental Protection Agency, Washington, DC, July 12-13, 2006. |
R830898 (2005) |
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| Proceedings | Lowry G, Tilton RD, Sholl D, Majetich S, Matyjaszewski K, Redden GD, Meakin P, Rollins HW. Transport, targeting, and applications of metallic functional nanoparticles for degradation of DNAPL chlorinated organic solvents. In: Proceedings of the 227th American Chemical Society National Meeting, Anaheim, CA, March 31, 2004, Vol. 44, No. 1, pp. 488-493. |
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| Proceedings | Lowry G. Nanoiron in the subsurface: how far will it go and how does it change? In: Proceedings of the U.S. EPA Workshop on Nanotechnology for Site Remediation, Department of Commerce, Washington, DC: U.S. Environmental Protection Agency, October 20-21, 2005. |
R830898 (Final) |
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| Proceedings | Phenrat T, Liu Y, Kim H-J, Saleh N, Sirk K, Tilton RD, Lowry GV. Effect of adsorbed polyelectrolytes on TCE dechlorination and product distribution by Fe0/Fe-oxide nanoparticles. In: Proceedings of the Division of Environmental Chemistry for the 233rd ACS National Meeting, Chicago, IL March 25-29, 2007. |
R830898 (Final) |
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| Proceedings | Saleh NB, Sirk K, Sarbu T, Tilton RD, et al. Transport and DNAPL targeting of polyelectrolyte-and surfactant-modified nanoiron. In: Proceedings of the Environmental Chemistry Division, 230h American Chemical Society National Meeting, Washington, DC, August 28-September 1, 2005. |
R830898 (2005) R830898 (Final) |
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The perspectives, information and conclusions conveyed in research project abstracts, progress reports, final reports, journal abstracts and journal publications convey the viewpoints of the principal investigator and may not represent the views and policies of ORD and EPA. Conclusions drawn by the principal investigators have not been reviewed by the Agency.