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METROPOLITAN-SCALE TRANSPORT AND DISPERSION FROM THE NEW YORK WORLD TRADE CENTER FOLLOWING SEPTEMBER 11, 2001. PART II: AN APPLICATION OF THE CALPUFF PLUME MODEL
Citation:
GILLIAM, R. C., A. H. HUBER, AND S. RAMAN. METROPOLITAN-SCALE TRANSPORT AND DISPERSION FROM THE NEW YORK WORLD TRADE CENTER FOLLOWING SEPTEMBER 11, 2001. PART II: AN APPLICATION OF THE CALPUFF PLUME MODEL. PURE & APPLIED GEOPHYSICS. Springer, New York, NY, 162(10):2005-2028, (2005).
Impact/Purpose:
The objective of this task is to improve EPA's ability to accurately predict the concentrations and deposition of air pollutants in the atmosphere that are known or suspected to cause cancer or other serious health effects to humans, or adverse environmental effects. It is an essential component of EPA's National Air Toxics Assessment (NATA), which seeks to identify and quantify the concentrations and sources of those hazardous air pollutants which are of greatest potential concern, in terms of contribution to population risk. It is a major contributor to NERL's Air Toxics Research Program.
"Air toxics" or "hazardous air pollutants" (HAPs) is a category that covers a large variety of chemicals, which range from relatively non reactive to extremely reactive; can exist in the gas, aqueous, and/or particle phases; display a large range of volatilities; experience varying deposition velocities, including in some cases revolatilization; and are emitted from a wide variety of sources at a large variety of different scales. In addition, concentrations of air toxics are needed by regulators for both short (days) as well as long (up to a year) time scales. These requirements challenge our current capabilities in air quality models far beyond the needs for other pollutants, such as ozone. The specific work being done under this task involves 1.) developing and testing chemical mechanisms which are appropriate for describing the chemistry of air toxics; 2.) incorporating these chemical and physical mechanisms into EPA's CMAQ modeling system and applying the model at a variety of scales; and 3.) developing the methods for using models to predict HAPs concentrations at subgrid or neighborhood scales; and 4.) using these tools to assess the magnitude and variability of concentrations to which urban populations are exposed.
Description:
Following the collapse of the New York World Trade Center (WTC) towers on September 11, 2001, Local, State, and Federal agencies initiated numerous air monitoring activities to better understand the ongoing impacts of emissions from the disaster. The collapse of the World Trade Center towers and associated fires that lasted for several weeks resulted at times in a noticeable plume of material that was dispersed around the Metropolitan New York City (NYC) area. In general, the plume was only noticeable for a short period of time following September 11, and only apparent close to the World Trade Center site. A study of the estimated pathway, which the plume of WTC material would likely follow, was completed to support the United States Environmental Protection Agency's 2002 initial exposure assessments. In this study, the WTC emissions were simulated using the CALMET-CALPUFF model in order to examine the general spatial and temporal dispersion patterns over NYC. This paper presents the results of the CALPUFF plume model in terms of plume dilution and location, since the exact source strength remains unknown. Independent observations of PM2.5 are used to support the general dispersion features calculated by the model. Results indicate that the simulated plume matched well with an abnormal increase (600-1000% of normal) in PM2.5 two nights after the WTC collapse as the plume rotated north to southeast, towards parts of NYC. Very little if any evidence of the plume signature was noted during a similar flow scenario a week after September 11. This leads to the conclusion that other than areas within a few kilometers from the WTC site, the PM2.5 plume was not observable over NYC's background concentration after the first few days.