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Records 26 to 50 of 508

Yields and molecular composition of gas-phase and secondary organic aerosol from the photooxidation of the volatile consumer product benzyl alcohol: formation of highly oxygenated and hydroxy nitro-aromatic compounds
(JOURNAL) [Published : Apr 19, 2023]
Recently, volatile chemical products (VCPs) have been increasingly recognized as important precursors for secondary organic aerosol (SOA) and ozone in urban areas. However, their atmospheric chemistry, physical transformation, and their impact on climate, environment and human he...
Associations of Air Pollution and Pediatric Asthma in Cleveland, Ohio
(JOURNAL) [Published : Sep 16, 2021]
Air pollution has been associated with poor health outcomes and continues to be a risk factor for respiratory health in children. While higher particulate matter (PM) levels are associated with increased frequency of symptoms, lower lung function, and increase airway inflammation...
Sensitivity of Riparian Buffer Designs to Climate Change—Nutrient and Sediment Loading to Streams: A Case Study in the Albemarle-Pamlico River Basins (USA) Using HAWQS
(JOURNAL) [Published : Nov 09, 2021]
Riparian buffer zones (RBZs) provide multiple benefits to watershed ecosystems. We aimed to conduct an extensive sensitivity analysis of the RBZ designs to climate change nutrient and sediment loadings to streams. We designed 135 simulation scenarios starting with the six baselin...
Improving the Characterization of the Natural Emissions in CMAQ
(JOURNAL) [Published : Oct 01, 2021]
The air quality of any given location is the result of complex interactions between meteorology and emissions through dynamical, physical, chemical, and photochemical processes. Of the many sources of air pollution, naturally produced emissions such as nitric oxide (NO) from soil...
Research Needed to Improve Air Quality Modeling: Recommendations from a 2022 Workshop
(JOURNAL) [Published : Jun 02, 2023]
The Coordinating Research Council (CRC) and the California Air Resources Board (CARB) co-sponsored an Air Quality Research Needs Workshop that was held November 8 and 9, 2022, on campus at the University of California, Davis. The workshop attracted over 60 attendees, including re...
Shifts in the Composition of Nitrogen Deposition in the Conterminous United States are Discernable in Stream Chemistry.
(JOURNAL) [Published : Jul 10, 2023]
This paper evaluates the relationships between recent shifts in the form (oxidized vs. reduced) of N deposition and watershed and stream chemistry by coupling estimates of N deposition with stream measurements from the U.S. EPA National Rivers and Streams Assessment (NRSA; three ...
Synthesis of lichen response to gaseous nitrogen: Ammonia versus nitrogen dioxide
(JOURNAL) [Published : Oct 10, 2022]
The dominant chemical species of nitrogen pollution emitted to the atmosphere in the U.S. and Europe is shifting from oxidized nitrogen (NOY) from combustion of fossil fuels to reduced nitrogen (NHX) from agricultural animal waste and fertilizer applications. Does it matter ...
Protection of forest ecosystems in the eastern United States from elevated atmospheric deposition of sulfur and nitrogen: A comparison of steady-state and dynamic model results
(JOURNAL) [Published : Dec 16, 2022]
Critical loads (CLs) and target loads (TLs) of atmospheric deposition of sulfur (S) and nitrogen (N) specify the thresholds of air pollution above which damage to ecosystems is expected to occur and are used to inform environmental regulation and natural resource management. Mode...
Major point and nonpoint sources of nutrient pollution to surface water have declined throughout the Chesapeake Bay watershed
(JOURNAL) [Published : May 22, 2022]
Understanding drivers of water quality in local watersheds is the first step for implementing targeted restoration practices. Nutrient inventories can inform water quality management decisions by succinctly communicating shifts in nitrogen (N) and phosphorus (P) balances over spa...
A sensitivity analysis of a human exposure model using the Sobol method
(JOURNAL) [Published : Nov 01, 2022]
The Air Pollutants Exposure Model (APEX) is a stochastic population-based inhalation exposure model which (along with its earlier version called pNEM) has been used by the U.S. Environmental Protection Agency (EPA) for over 30 years for assessment of human exposure to airborne po...
The contribution of the neuroendocrine system to adaption after repeated daily ozone exposure in rats
(JOURNAL) [Published : Jul 15, 2022]
Ozone-induced lung injury/inflammation dissipates despite continued exposure for 3 or more days; however, the mechanisms of adaptation/habituation remain unclear. Since ozone effects are mediated through adrenal-derived stress hormones, which also regulate longevity of centrally-...
Beyond Particulate Matter Mass: Heightened Levels of Lead and Other Pollutants Associated with Destructive Fire Events in California
(JOURNAL) [Published : Oct 18, 2022]
Abstract: As the climate warms, wildfires are increasing in size and intensity, posing a risk to human health and sensitive ecosystems. Studies have reported on particulate matter (PM) in wildfire smoke; however, the chemicals associated with PM, including toxic metals, have rece...
Empirical nitrogen and sulfur critical loads of U.S. tree species and their uncertainties with machine learning
(JOURNAL) [Published : Oct 08, 2022]
Critical loads (CLs) of atmospheric deposition for nitrogen and sulfur are used to support decision making related to air regulation and land management. Frequently CLs are calculated CLs using empirical methods, and the certainty of the results from these methods depends on thei...
Nitrogen and Sulfur Deposition Reductions Projected to Partially Restore Forest Soil Conditions in the US Northeast, While Understory Composition Continues to Shift with Future Climate Change
(JOURNAL) [Published : Sep 05, 2022]
We used a dynamic soil-vegetation model (ForSAFE-Veg) to simulate responses to future scenarios of atmospheric deposition and climate change across 23 Northeastern hardwood stands. Specifically, we simulated soil percent base saturation, acid neutralizing capacity (ANC), nitrate ...
Modeled vegetation community trajectories: Effects from climate change, atmospheric nitrogen deposition, and soil acidification recovery
(JOURNAL) [Published : Jul 28, 2022]
Forest understory plant communities in the United States are diverse and often sensitive to changes in climate and atmospheric inputs of nitrogen (N) caused by air pollution. Recently, understory vegetation response functions (expressed as Probability of Occurrence of Plant Speci...
Modeling Streamflow and Water Quality Sensitivity to Climate Change and Urban Development in 20 U.S. Watersheds.
(JOURNAL) [Published : Oct 01, 2015]
Watershed modeling in 20 large, United States (U.S.) watersheds addresses gaps in our knowledge of streamflow, nutrient (nitrogen and phosphorus), and sediment loading sensitivity to mid-21st Century climate change and urban/residential development scenarios. Use of a consistent ...
Declines and peaks in NO2 pollution during the multiple waves of the COVID-19 pandemic in the New York metropolitan area
(JOURNAL) [Published : Feb 22, 2022]
The COVID-19 pandemic created an extreme natural experiment in which sudden changes in human behavior and economic activity resulted in significant declines in nitrogen oxide (NOx) emissions, immediately after strict lockdowns were imposed. Here we examined the impact of multiple...
Boundary layer versus free tropospheric submicron particle formation: A case study from NASA DC-8 observations in the Asian continental outflow during the KORUS-AQ campaign
(JOURNAL) [Published : Dec 31, 2021]
In this study, we contrasted major secondary inorganic species and processes responsible for submicron particle formation (SPF) events in the boundary layer (BL) and free troposphere (FT) over the Korean Peninsula during Korea-United States Air Quality (KORUS-AQ) campaign (May-Ju...
The Role of Hepatic Vagal Tone in Ozone-induced Metabolic Dysfunction in the Liver
(JOURNAL) [Published : Jun 01, 2021]
  Air pollution has been associated with metabolic diseases and hepatic steatosis-like changes. We have shown that ozone alters liver gene expression for metabolic processes through neuroendocrine activation. This study aimed to further characterize ozone-induced changes and...
Disinfection Byproducts in Chlorinated or Brominated Swimming Pools and Spas: Role of Brominated DBPs and Association with Mutagenicity
(JOURNAL) [Published : Jul 01, 2022]
Although the health benefits of swimming are well-documented, health effects such as asthma and bladder cancer are linked to disinfection by-products (DBPs) in pool water.  DBPs are formed from the reaction of disinfectants such as chlorine (Cl) or bromine (Br) with organics...
Comprehensive evaluations of diurnal NO2 measurements during DISCOVER-AQ 2011: effects of resolution-dependent representation of NOx emissions
(JOURNAL) [Published : Jul 23, 2021]
Nitrogen oxides (NOx=NO2NO2) play a crucial role in the formation of ozone and secondary inorganic and organic aerosols, thus affecting human health, global radiation budget, and climate. The diurnal and spatial variations in NO2 are functions of emissions, advection, deposition,...
Changes in ozone chemical sensitivity in the U.S. from 2007 to 2016
(JOURNAL) [Published : Dec 16, 2021]
Anthropogenic nitrogen oxide (NOx) and volatile organic compound (VOC) emissions in the U.S. have declined substantially over the last decade, altering the NOx-VOC chemistry and ozone (O3) production characteristics of many areas. In this work we use multiple air quality analysis...
Impacts of lake breeze meteorology on ozone gradient observations along Lake Michigan shorelines in Wisconsin
(JOURNAL) [Published : Jan 15, 2022]
Daytime onshore lake breezes are a critical factor controlling ozone abundance at coastal sites around Lake Michigan. Coastal counties along the western shore of Lake Michigan have historically observed high ozone episodes dating to the 1970s. We classified ozone episode days bas...
Characterization of ground-based atmospheric pollution and meteorology sampling stations during the Lake Michigan Ozone Study 2017
(JOURNAL) [Published : Jul 03, 2021]
The Lake Michigan Ozone Study 2017 (LMOS 2017) in May and June 2017 enabled study of transport, emissions, and chemical evolution related to ozone air pollution in the Lake Michigan airshed. Two highly instrumented ground sampling sites were part of a wider sampling strategy of a...
4D-Var Inversion of European NH3 Emissions Using CrIS NH3 Measurements and GEOS-Chem Adjoint With Bi-Directional and Uni-Directional Flux Schemes
(JOURNAL) [Published : May 16, 2022]
We conduct the first 4D-Var inversion of NH3 accounting for NH3 bi-directional flux, using CrIS satellite NH3 observations over Europe in 2016. We find posterior NH3 emissions peak more in springtime than prior emissions at continental to national scales, and ...