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The Effects of Global Change upon United States Air Quality
Citation:
Gonzalez-Abraham, R., S. Chung, J. Avise, B. Lamb, E. Salathe, Chris Nolte, Dan Loughlin, A. Guenther, C. Wiedinmyer, T. Duhl, Y. Zhang, AND D. Streets. The Effects of Global Change upon United States Air Quality. Atmospheric Chemistry and Physics Discussions. Copernicus Gesellschaft mbH, Gottingen, Germany, 15:12645-12665, (2015).
Impact/Purpose:
The National Exposure Research Laboratory’s Atmospheric Modeling Division (AMAD) conducts research in support of EPA’s mission to protect human health and the environment. AMAD’s research program is engaged in developing and evaluating predictive atmospheric models on all spatial and temporal scales for forecasting the Nation’s air quality and for assessing changes in air quality and air pollutant exposures, as affected by changes in ecosystem management and regulatory decisions. AMAD is responsible for providing a sound scientific and technical basis for regulatory policies based on air quality models to improve ambient air quality. The models developed by AMAD are being used by EPA, NOAA, and the air pollution community in understanding and forecasting not only the magnitude of the air pollution problem, but also in developing emission control policies and regulations for air quality improvements.
Description:
To understand more fully the effects of global changes on ambient concentrations of ozone and particulate matter with aerodynamic diameter smaller than 2.5 μm (PM2.5) in the US, we conducted a comprehensive modeling effort to evaluate explicitly the effects of changes in climate, biogenic emissions, land use, and global/regional anthropogenic emissions on ozone and PM2.5 concentrations and composition. Results from the ECHAM5 global climate model driven with the A1B emission scenario from the Intergovernmental Panel on Climate Change (IPCC) were downscaled using the Weather Research and Forecasting (WRF) model to provide regional meteorological fields. We developed air quality simulations using the Community Multiscale Air Quality Model (CMAQ) chemical transport model for two nested domains with 220 km and 36 km horizontal grid cell resolution for a semi-hemispheric domain and a continental United States (US) domain, respectively. The semi-hemispheric domain was used to evaluate the impact of projected Asian emissions changes on US air quality. WRF meteorological fields were used to calculate current (2000s) and future (2050s) biogenic emissions using the Model of Emissions of Gases and Aerosols from Nature (MEGAN). For the semi-hemispheric domain CMAQ simulations, present-day global emissions inventories were used and projected to the 2050s based on the IPCC A1B scenario. Regional anthropogenic emissions were obtained from the US Environmental Protection Agency National Emission Inventory 2002 (EPA NEI2002) and projected to the future using the MARKet ALlocation (MARKAL) energy system model assuming a business as usual scenario that extends current decade emission regulations through 2050. Our results suggest that daily maximum 8 hour average ozone (DM8O) concentrations will increase in a range between 2 to 12 ppb across most of the continental US, with the highest increase in the South, Central, and Midwest regions of the US, due to increases in temperature, enhanced biogenic emissions, and changes in land use. The effects of these factors are only partially offset by reductions in DM8O associated with decreasing US anthropogenic emissions. Increases in PM2.5 levels between 2 and 4 μg m-3 in the Northeast, Southeast, and South regions are mostly a result of enhanced biogenic emissions and land use changes. Little change in PM2.5 in the Central, Northwest, and Southwest regions was found, even when PM precursors are reduced with regulatory curtailment. Changes in temperature, relative humidity, and boundary conditions shift the composition but do not alter overall PM2.5 mass concentrations.
URLs/Downloads:
THE EFFECTS OF GLOBAL CHANGE UPON UNITED STATES AIR QUALITY.PDF (PDF, NA pp, 2382.366 KB, about PDF)Atmospheric Chemistry and Physics
